%0 Journal Article %1 ADMA:ADMA201703852 %A Jiang, Qi %A Chu, Zema %A Wang, Pengyang %A Yang, Xiaolei %A Liu, Heng %A Wang, Ye %A Yin, Zhigang %A Wu, Jinliang %A Zhang, Xingwang %A You, Jingbi %D 2017 %J Advanced Materials %K 21% efficiency perovskite planar %P n/a--n/a %R 10.1002/adma.201703852 %T Planar-Structure Perovskite Solar Cells with Efficiency beyond 21% %U http://dx.doi.org/10.1002/adma.201703852 %X Low temperature solution processed planar-structure perovskite solar cells gain great attention recently, while their power conversions are still lower than that of high temperature mesoporous counterpart. Previous reports are mainly focused on perovskite morphology control and interface engineering to improve performance. Here, this study systematically investigates the effect of precise stoichiometry, especially the PbI2 contents on device performance including efficiency, hysteresis and stability. This study finds that a moderate residual of PbI2 can deliver stable and high efficiency of solar cells without hysteresis, while too much residual PbI2 will lead to serious hysteresis and poor transit stability. Solar cells with the efficiencies of 21.6% in small size (0.0737 cm2) and 20.1% in large size (1 cm2) with moderate residual PbI2 in perovskite layer are obtained. The certificated efficiency for small size shows the efficiency of 20.9%, which is the highest efficiency ever recorded in planar-structure perovskite solar cells, showing the planar-structure perovskite solar cells are very promising.

@article{ADMA:ADMA201703852, abstract = {Low temperature solution processed planar-structure perovskite solar cells gain great attention recently, while their power conversions are still lower than that of high temperature mesoporous counterpart. Previous reports are mainly focused on perovskite morphology control and interface engineering to improve performance. Here, this study systematically investigates the effect of precise stoichiometry, especially the PbI2 contents on device performance including efficiency, hysteresis and stability. This study finds that a moderate residual of PbI2 can deliver stable and high efficiency of solar cells without hysteresis, while too much residual PbI2 will lead to serious hysteresis and poor transit stability. Solar cells with the efficiencies of 21.6% in small size (0.0737 cm2) and 20.1% in large size (1 cm2) with moderate residual PbI2 in perovskite layer are obtained. The certificated efficiency for small size shows the efficiency of 20.9%, which is the highest efficiency ever recorded in planar-structure perovskite solar cells, showing the planar-structure perovskite solar cells are very promising.}, added-at = {2017-11-06T11:47:05.000+0100}, author = {Jiang, Qi and Chu, Zema and Wang, Pengyang and Yang, Xiaolei and Liu, Heng and Wang, Ye and Yin, Zhigang and Wu, Jinliang and Zhang, Xingwang and You, Jingbi}, biburl = {https://www.bibsonomy.org/bibtex/258b4ebd12a68f7b8097b4cce865eede3/fabianopkm}, description = {Planar-Structure Perovskite Solar Cells with Efficiency beyond 21% - Jiang - 2017 - Advanced Materials - Wiley Online Library}, doi = {10.1002/adma.201703852}, interhash = {6398bc335c963d240c52a483eef3575a}, intrahash = {58b4ebd12a68f7b8097b4cce865eede3}, issn = {1521-4095}, journal = {Advanced Materials}, keywords = {21% efficiency perovskite planar}, pages = {n/a--n/a}, timestamp = {2017-11-06T11:47:05.000+0100}, title = {Planar-Structure Perovskite Solar Cells with Efficiency beyond 21%}, url = {http://dx.doi.org/10.1002/adma.201703852}, year = 2017 }