Abstract
We present evidence that the cosmological mean metallicity of neutral atomic
hydrogen gas shows a sudden decrease at $z>4.7$ down to $< Z
>=-2.03^+0.09_-0.11$, which is $6\sigma$ deviant from that predicted by a
linear fit to the data at lower redshifts. This measurement is made possible by
the chemical abundance measurements of 8 new damped Ly-$\alpha$ (DLA) systems
at $z>4.7$ observed with the Echellette Spectrograph and Imager on the Keck II
telescope, doubling the number of measurements at $z>4.7$ to 16. The sudden
decrease in metallicity is possibly due to the lower ultra-violet radiation
field and higher density at high redshift increasing the neutral fraction of
gas inside halos, such as cold flows. This would result in a new population of
presumably lower metallicity DLAs, with an increased contribution to the DLA
population at higher redshifts resulting in a reduced mean metallicity. While
the comoving metal mass density of DLAs, $\rho_metals(z)_DLA$, is
flat out to $z\sim4.3$, there is evidence of a possible decrease at $z>4.7$.
Such a decrease is expected, as otherwise most of the metals from star-forming
galaxies would reside in DLAs by $z\sim6$. While the metallicity is decreasing
at high redshift, the contribution of DLAs to the total metal budget of the
universe increases with redshift, with DLAs at $z\sim4.3$ accounting for
$\sim20$% as many metals as produced by Lyman break galaxies.
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