%0 Journal Article %1 C3FD90021E %A Stolow, Albert %D 2013 %I The Royal Society of Chemistry %J Faraday Discuss. %K chemistry dynamics reaction review unread %N 0 %P 9-32 %R 10.1039/C3FD90021E %T The three pillars of photo-initiated quantum molecular dynamics %U http://dx.doi.org/10.1039/C3FD90021E %V 163 %X Studies of the interaction of light with matter, based on spectroscopy and diffraction, yielded a microscopic view of nature. The detailed structure of molecules and solids emerged from this effort and led to many of the advances of the 20th century, with the 'structure-function' paradigm being perhaps paramount. This static view of Nature is a necessary but insufficient advance and, in the 21st century, we will need to develop microscopic yet dynamical views of Nature. We consider here issues in Photo-initiated Quantum Molecular Dynamics raised by Faraday Discussions 163, in the context of three main categories or 'pillars' of light-matter interaction: energy/time, phase/coherence, intensity.

@article{C3FD90021E, abstract = {Studies of the interaction of light with matter{,} based on spectroscopy and diffraction{,} yielded a microscopic view of nature. The detailed structure of molecules and solids emerged from this effort and led to many of the advances of the 20th century{,} with the {'}structure-function{'} paradigm being perhaps paramount. This static view of Nature is a necessary but insufficient advance and{,} in the 21st century{,} we will need to develop microscopic yet dynamical views of Nature. We consider here issues in Photo-initiated Quantum Molecular Dynamics raised by Faraday Discussions 163{,} in the context of three main categories or {'}pillars{'} of light-matter interaction: energy/time{,} phase/coherence{,} intensity.}, added-at = {2013-07-28T14:50:56.000+0200}, author = {Stolow, Albert}, biburl = {https://www.bibsonomy.org/bibtex/2860ec97c05ac936a08c4b9fc6a4ded32/drmatusek}, doi = {10.1039/C3FD90021E}, interhash = {b05a901a63ca5c781628fe4ef955f5dc}, intrahash = {860ec97c05ac936a08c4b9fc6a4ded32}, journal = {Faraday Discuss.}, keywords = {chemistry dynamics reaction review unread}, month = jul, number = 0, pages = {9-32}, publisher = {The Royal Society of Chemistry}, timestamp = {2013-07-28T14:50:57.000+0200}, title = {The three pillars of photo-initiated quantum molecular dynamics}, url = {http://dx.doi.org/10.1039/C3FD90021E}, volume = 163, year = 2013 }