An electronic solid with itinerant carriers and localized magnetic moments represents a paradigmatic strongly correlated system. The electrical transport properties associated with the itinerant carriers, as they scatter off these local moments, have been scrutinized across a number of materials. Here, we analyze the transport characteristics associated with ultraclean PdCrO2?a quasi-two-dimensional material consisting of alternating layers of itinerant Pd-electrons and Mott-insulating CrO2 layers?which shows a pronounced regime of T-linear resistivity over a wide range of intermediate temperatures. By contrasting these observations to the transport properties in a closely related material PdCoO2, where the CoO2 layers are band-insulators, we can rule out the traditional electron?phonon interactions as being responsible for this interesting regime. We propose a previously ignored electron-magneto-elastic interaction between the Pd-electrons, the Cr local moments and an out-of-plane phonon as the main scattering mechanism that leads to the significant enhancement of resistivity and a T-linear regime in PdCrO2 at temperatures far in excess of the magnetic ordering temperature. We suggest a number of future experiments to confirm this picture in PdCrO2 as well as other layered metallic/Mott-insulating materials.
%0 Journal Article
%1 mendezvalderrama2023tlinear
%A Mendez-Valderrama, J. F.
%A Tulipman, Evyatar
%A Zhakina, Elina
%A Mackenzie, Andrew P.
%A Berg, Erez
%A Chowdhury, Debanjan
%D 2023
%I Proceedings of the National Academy of Sciences
%J Proc. Natl. Acad. Sci.
%K b
%N 36
%P e2305609120--
%R 10.1073/pnas.2305609120
%T T-linear resistivity from magneto-elastic scattering: Application to PdCrO$_2$
%U https://doi.org/10.1073/pnas.2305609120
%V 120
%X An electronic solid with itinerant carriers and localized magnetic moments represents a paradigmatic strongly correlated system. The electrical transport properties associated with the itinerant carriers, as they scatter off these local moments, have been scrutinized across a number of materials. Here, we analyze the transport characteristics associated with ultraclean PdCrO2?a quasi-two-dimensional material consisting of alternating layers of itinerant Pd-electrons and Mott-insulating CrO2 layers?which shows a pronounced regime of T-linear resistivity over a wide range of intermediate temperatures. By contrasting these observations to the transport properties in a closely related material PdCoO2, where the CoO2 layers are band-insulators, we can rule out the traditional electron?phonon interactions as being responsible for this interesting regime. We propose a previously ignored electron-magneto-elastic interaction between the Pd-electrons, the Cr local moments and an out-of-plane phonon as the main scattering mechanism that leads to the significant enhancement of resistivity and a T-linear regime in PdCrO2 at temperatures far in excess of the magnetic ordering temperature. We suggest a number of future experiments to confirm this picture in PdCrO2 as well as other layered metallic/Mott-insulating materials.
@article{mendezvalderrama2023tlinear,
abstract = {An electronic solid with itinerant carriers and localized magnetic moments represents a paradigmatic strongly correlated system. The electrical transport properties associated with the itinerant carriers, as they scatter off these local moments, have been scrutinized across a number of materials. Here, we analyze the transport characteristics associated with ultraclean PdCrO2?a quasi-two-dimensional material consisting of alternating layers of itinerant Pd-electrons and Mott-insulating CrO2 layers?which shows a pronounced regime of T-linear resistivity over a wide range of intermediate temperatures. By contrasting these observations to the transport properties in a closely related material PdCoO2, where the CoO2 layers are band-insulators, we can rule out the traditional electron?phonon interactions as being responsible for this interesting regime. We propose a previously ignored electron-magneto-elastic interaction between the Pd-electrons, the Cr local moments and an out-of-plane phonon as the main scattering mechanism that leads to the significant enhancement of resistivity and a T-linear regime in PdCrO2 at temperatures far in excess of the magnetic ordering temperature. We suggest a number of future experiments to confirm this picture in PdCrO2 as well as other layered metallic/Mott-insulating materials.},
added-at = {2023-12-18T11:01:57.000+0100},
author = {Mendez-Valderrama, J. F. and Tulipman, Evyatar and Zhakina, Elina and Mackenzie, Andrew P. and Berg, Erez and Chowdhury, Debanjan},
biburl = {https://www.bibsonomy.org/bibtex/237ba6fbb83f260a1490c95a9412e78ca/ctqmat},
comment = {doi: 10.1073/pnas.2305609120},
day = 28,
doi = {10.1073/pnas.2305609120},
interhash = {90d37f5a4127268fdda16e651e1bce06},
intrahash = {37ba6fbb83f260a1490c95a9412e78ca},
journal = {Proc. Natl. Acad. Sci.},
keywords = {b},
month = {08},
number = 36,
pages = {e2305609120--},
publisher = {Proceedings of the National Academy of Sciences},
timestamp = {2023-12-18T11:01:57.000+0100},
title = {T-linear resistivity from magneto-elastic scattering: Application to PdCrO$_\mathbf{2}$},
url = {https://doi.org/10.1073/pnas.2305609120},
volume = 120,
year = 2023
}