Article,

Field-induced magnetic transitions in the highly anisotropic ferrimagnet ErFe$_5$Al$_7$ studied by high-field x-ray magnetic dichroism

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Phys. Rev. B, 109 (9): 094404 (Mar 5, 2024)
DOI: 10.1103/PhysRevB.109.094404

Abstract

We present a comprehensive study of the magnetic properties of the strongly anisotropic ferrimagnet $ErFe_5Al_7$ in pulsed magnetic fields up to 30 T applied along the hard magnetization axis within the basal plane of the tetragonal lattice around the compensation temperature ($T_comp$). Macroscopic measurements showed two anomalies at about 8 T and 25 T in a small temperature range around $T_comp$. High-field x-ray magnetic circular dichroism (XMCD) data at the Er $M_5$- and the Fe $L_3$-edge resonances provide insight into the element-selective magnetization processes, revealing a coherent rotation of Er $4f$ and Fe $3d$ moments, with stepwise jumps including an unexpected one from an easy to a hard magnetization axis. XMCD at the Er $L_3$-edge resonance elucidates the role of Er $5d$ electrons in coupling the Er $4f$ and the Fe $3d$ moments. Finally, an in-plane anisotropy constant was evaluated from a simulation of the magnetization process at temperatures well below $T_comp$ using a two-sublattice model.

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