Abstract
A formula for frequency-dependent optical second-harmonic susceptibilities
for insulating crystals, including local-field corrections, is presented.
In analogy to a formula given previously for the static limit, the
formula is analyzed in terms of ''virtual electron'' (ccv) and ''virtual
hole'' (vvc) terms to obtain a numerically stable form. Numerical
results for GaP and GaAs agree with most of the experimental values
suggested in a recent review article by Roberts. Miller's DELTA(M)
is predicted to vary by 13% from the laser lines at 10.6 to 1.32
mum for GaP.
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